000 02515cam a2200325 a 4500
003 EG-GiCUC
005 20250223032645.0
008 201219s2020 ua f m 000 0 eng d
040 _aEG-GiCUC
_beng
_cEG-GiCUC
041 0 _aeng
049 _aDeposite
097 _aPh.D
099 _aCai01.12.10.Ph.D.2020.Ma.S
100 0 _aMarwa Maher Abdelmohsen Bayoumi
245 1 0 _aSynthesis of some new heterocyclic compounds from nitrile derivatives /
_cMarwa Maher Abdel Mohsen Bayoumi ; Supervised Sanaa Osman Abdallah
246 1 5 _aتشييد بعض المركبات غير المتجانسة الحلقة الجديدة من مشتقات النيترين
260 _aCairo :
_bMarwa Maher Abdel Mohsen Bayoumi ,
_c2020
300 _a222 P. ;
_c25cm
502 _aThesis (Ph.D.) - Cairo University - Faculty of Science - Department of Organic Chemistry
520 _aThe starting N,N-bis(cyanoacetyl)hydrazine 3 was prepared by the reaction of cyanoacetic acid hydrazide 1 and 3-(3 ,5-dimethyl-1H-pyrazol-1-yl)-3- oxopropanenitrile 2. Condensation of compound 3 with each of aromatic aldehydes 4a-k, o-hydroxybenzaldehydes 8a,b and azosalicylaldehydes 12a-e under grind stone method afforded the respective arylmethylene derivatives Sak, his-coumarin derivatives lla,b and 15a-e, respectively. Coupling of 3 with aryldiazonium chlorides gave arylhydrazono derivatives 17a-e. Also , antimicrobial activity for some new products, enzyme inhibition and agarose gel electrophoresis were investigated. Next, malononitrile considered as the starting material to prepare 5-amino-3- (cyanomethyl)-1-phenyl-lH-pyrazole-4-carbonitrile 20. Acid hydrolysis of compound 20 gave 3-amino-2-phenyl-2,7-dihydro-4H-pyrazolo[ 4,3-c ]pyridine- 4,6(5H)-dione 39. Condensation of each of 20 and 39 with various aromatic aldehydes afforded the corresponding arylmethylenes 23a-i and 40a-I, respectively. Coupling of 39 with aryldiazonium chlorides led to formation of arylhydrazono derivatives 53a-e.Moroever, acetylation of 39 yielded the Nacetyl derivative 43. The anticancer activity of some of the newly synthesized compounds was investigated. Also, molecular docking study was performed
530 _aIssued also as CD
653 4 _aAntimicrobial activity
653 4 _aBis-coumarins
653 4 _aN,N-bis( cyanoacetyl)hydrazine
700 0 _aSanaa Osman Abdallah ,
_eSupervisor
856 _uhttp://172.23.153.220/th.pdf
905 _aNazla
_eRevisor
905 _aShimaa
_eCataloger
942 _2ddc
_cTH
999 _c79264
_d79264